lazyf3 When the OS isn't on Raid 0, you can probably just follow https://wiki.archlinux.org/index.php/RAID#Installation . But warnings ahead I never set up a Raid 0 on Solus.
Yes I think there won't be a big improvement, but don't take my words for granted. Sometimes it's just better to try it out yourself instead of reading a comment from a random dude in the internet 😉
Edit: Maybe easier then setting up mdadm would be to use btrfs for your gaming partition:
mkfs.btrfs -d raid0 /dev/yourdevice1 /dev/yourdevice2